4.結(jié)論

首次將Langmuir-Schaefer方法用于DEAs電極的制備。將多壁碳納米管和聚（烷基噻吩）結(jié)合在一起，在空氣-水界面形成穩(wěn)定的單分子膜，然后使用Langmuir-Schaefer技術(shù)將其轉(zhuǎn)移到PDMS膜上。單層電極由嵌入鉑單層中的互連多壁碳納米管網(wǎng)絡(luò)組成，其中鉑賦予機(jī)械性能，而多壁碳納米管確保系統(tǒng)的導(dǎo)電性。復(fù)合單分子膜可拉伸，導(dǎo)電率高達(dá)100%(～20 MΩ/0%應(yīng)變時(shí)，～5 GΩ/在100%應(yīng)變下）。使用LS方法制作圖案化超薄可拉伸電極，可以制作具有1.4μm厚PDMS介電膜的薄DEA。僅在100V下，該DEA達(dá)到4.0%線性應(yīng)變。與DEAs通常需要的kV驅(qū)動(dòng)電壓相比，這種低工作電壓為DEAs開辟了新的應(yīng)用領(lǐng)域。我們?cè)谶@里報(bào)告的LS電極是DEA在小于5V時(shí)產(chǎn)生全應(yīng)變的關(guān)鍵構(gòu)件：通過使用LS/LB技術(shù)制造彈性體和電極，將有可能制造多層DEA，其中所有層都是一個(gè)單分子厚度。這將是DEA技術(shù)的最終物理極限。

致謝

我們衷心感謝Jun Shintake博士、Matthias Imboden博士、Alexandre Poulin博士和Samuel Schlater先生的有益評(píng)論和討論。這項(xiàng)工作是由歐盟的地平線2020研究和創(chuàng)新計(jì)劃在瑪麗SK·OOOWSKA居里補(bǔ)助金協(xié)議，第64 1822-MICACT通過瑞士國(guó)家教育、研究和創(chuàng)新秘書處，以及瑞士國(guó)家科學(xué)基金會(huì)授予第200020號(hào)165993。

附錄A.補(bǔ)充數(shù)據(jù)

與本文相關(guān)的補(bǔ)充數(shù)據(jù)可在在線版本中找到，網(wǎng)址為https://doi.org/10.1016/j.snb.2018.01.145.

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